Розчинность водню у металах та їх сплавах
Анотація
Оглядовий матеріал розкриває питання щодо впливу домішок на фізичні властивості сплавів, а також про роль газів в процесах у сплавах. Встановлено, що наявність водню впливає на дифузію у сплавах, а гази значно впливають на термоелектрорушійну силу металів.
У роботі подан опис ефекту додавання третього елементу до бінарних систем, що може розширювати або звужувати область існування впорядкованої фази. Наведені приклади додавання домішки ванадію або молібдену в сплав заліза та хрому, що підвищує температуру впорядкування.
Виявлено, що гази можуть значно впливати на термоелектрорушійну силу металів та підвищувати твердість і зменшувати їх пластичність, а також викликати їхню хрупкість та розшарування. Показано, що водень (Н2) у сплавах (наприклад, у Fe-Ni та Au-Cu) впливає на дифузію та процеси атомного впорядкування. Також, мала концентрація водню, як домішки може змінювати електроопір сплавів (наприклад, у сплаві Pd-Au). Зазначено, що додавання третього елементу до бінарних систем може змінювати діаграму стану, що необхідно враховувати при вирішенні завдань з режимів термічної обробки сплавів, визначення умов фазової рівноваги і т.д.
У роботі розглянута залежність розчинності водню від температури в чистих металах (Cu, Fe та Al) та паказана її залежність у сплавах від концентрації домішкових металів, а також показана температурна залежність розчинності водню у сплавах Fe-V.
Вивчено зсув густини станів при різному розподілі домішкових атомів у сплаві при системі порядок-безлад, а також досліджена залежність густини станів неупорядкованих та впорядкованих твердих розчинів.
Вказана залежность відносної розчинності атомів, які впроваджуються в пори сплавів з ГЦК структурою (типу Cu3Au), з урахуванням розчинність від параметра χ, пропорційного мірі дальнього порядку в октаедричних та тетраедричних порах сплавів. Розглянута залежності відносної розчинності впроваджених атомів в октаедричних порах сплавів з ОЦК структурою (типу CuZn та Fe3Al).
Побудовані графіки залежності концентрації розчинених атомів домішок, від міри порядку для сплавів заміщення з ОЦК решіткою, де коефіцієнт М2 впровадженний не залежить від міри порядку.
Також вивчений вплив тиску на міру дальнього порядку, де його ступінь зменшується або збільшується, чи зменшується, а потім збільшується та навпаки (фазовий перехід порядок-безлад).
Не меньш важливим результатом є отримані залежності розчинності (с) від тиску (Р) в невпорядкованих та впорядкованих сплавах.
Посилання
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